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I do not think you can set it like that, but I just use the "F" key for zoom to fit since one hand is free.
this is a 2009 enhancement Brian. Double MMB zooms to fit in 09.
If you can't wait until SW2009, you can write a script using Autohotkey (free automation software). It can intercept a MMB double-click and do whatever scripted action you wish, including outputting the "f" key for fit to screen.